JOURNAL OF LIGHT INDUSTRY

CN 41-1437/TS  ISSN 2096-1553

6种香料在加热条件下的释放迁移及对气溶胶理化特性的影响

司晓喜,张凤梅,朱瑞芝,唐石云,杨继,刘春波,刘绍锋,崔华鹏

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司晓喜, 张凤梅, 朱瑞芝, 等. 6种香料在加热条件下的释放迁移及对气溶胶理化特性的影响[J]. 轻工学报, 2021, 36(5): 67-75. doi: 10.12187/2021.05.009
引用本文:司晓喜, 张凤梅, 朱瑞芝, 等. 6种香料在加热条件下的释放迁移及对气溶胶理化特性的影响[J]. 轻工学报, 2021, 36(5): 67-75.doi:10.12187/2021.05.009
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SI Xiaoxi, ZHANG Fengmei, ZHU Ruizhi, et al. Study on the release and migration of six flavourings under heating conditions and their effects on the physical and chemical properties of aerosols[J]. Journal of Light Industry, 2021, 36(5): 67-75. doi: 10.12187/2021.05.009
Citation:SI Xiaoxi, ZHANG Fengmei, ZHU Ruizhi, et al. Study on the release and migration of six flavourings under heating conditions and their effects on the physical and chemical properties of aerosols[J]. Journal of Light Industry, 2021, 36(5): 67-75.doi:10.12187/2021.05.009
shu

6种香料在加热条件下的释放迁移及对气溶胶理化特性的影响

  • 1. 云南中烟工业有限责任公司 技术中心/云南省烟草化学重点实验室, 云南 昆明 650031;

  • 2. 中国烟草总公司郑州烟草研究院, 河南 郑州 450001

    • 作者简介:司晓喜(1986-),男,云南省昆明市人,云南中烟工业有限责任公司高级工程师,主要研究方向为烟草和烟气化学.;

  • 基金项目:中国烟草总公司重大专项项目（110201901002（XX-02））；云南省科技厅科技项目（202001AU070005）；云南中烟工业有限责任公司科技项目（2020YL03）

  • 中图分类号:TS41+1;TQ656+.5;O551.3

Study on the release and migration of six flavourings under heating conditions and their effects on the physical and chemical properties of aerosols

  • 1. Technology Center, China Tobacco Yunnan Industrial Co., Ltd. /Key Lab of Tobacco Chemistry of Yunnan, Kunming 650031, China;

  • 2. Zhengzhou Tobacco Research Institute of CNTC, Zhengzhou 450001, China

  • Received Date:2021-05-14

    CLC number:TS41+1;TQ656+.5;O551.3

  • 摘要:采用吸烟机抽吸，结合GC-MS/MS和快速粒径仪检测，研究了6种香料在加热条件下向烟气气溶胶的迁移及对气溶胶理化特性的影响.实验结果表明：1）6种香料在350℃加热条件下均以原型蒸发为主.2）6种香料在加热抽吸时的释放迁移呈现不同特征，其中异戊酸异戊酯和2，3，5-三甲基吡嗪分布于烟气气溶胶粒相物和气相物中，其他4种香料均只分布于粒相物中；香叶醇和2-乙酰基吡咯向烟气气溶胶迁移的总迁移率为2.8%~8.1%，其余4种香料为17.6%~54.4%.3）与空白对照样相比，添加5%的L-薄荷醇或1%、2%的WS-23后，使烟碱、丙二醇和丙三醇向烟气气溶胶中的释放量降低了20%以上，在滤嘴段的截留量降低了10%以上.4）当L-薄荷醇添加量达5%时，气溶胶粒数浓度降低了28%、粒数中值直径（CMD）增大了8%.
    Abstract:The migration of six flavourings to smoke aerosols and their effects on the physical and chemical properties of aerosols under heating condition were studied by using a smoking machine, combined with GC-MS/MS and fast particulate spectrometer. The results showed that:1) The six flavourings were mainly evaporated by prototype at 350℃. 2) The release and migration of the six flavourings showed different characteristics under heating and suction conditions. Isoamyl isovalerate and 2,3,5-trimethylpyrazine were transferred to particle phase and gas phase of aerosol, while the other four flavourings were only transferred to particle phase of aerosol. The total migration rates of geraniol and 2-acetylpyrrole to smoke aerosol were 2.8%~8.1%, and the other four flavourings were 17.6%~54.4%. 3) Compared with the blank control, after adding 5% L-menthol or 1% and 2% WS-23, the release amount of nicotine, propylene glycol and glycerol from the tobacco materials to the aerosol was reduced by more than 20%, and their interception in the filter section was reduced by more than 10%. 4) When L-menthol was added to 5%, the particle number concentration decreased by 28% and count median diameter (CMD) increased by 8%.
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    司晓喜, 张凤梅, 朱瑞芝, 等. 6种香料在加热条件下的释放迁移及对气溶胶理化特性的影响[J]. 轻工学报, 2021, 36(5): 67-75. doi: 10.12187/2021.05.009
    引用本文:司晓喜, 张凤梅, 朱瑞芝, 等. 6种香料在加热条件下的释放迁移及对气溶胶理化特性的影响[J]. 轻工学报, 2021, 36(5): 67-75.doi:10.12187/2021.05.009
    shu
    SI Xiaoxi, ZHANG Fengmei, ZHU Ruizhi, et al. Study on the release and migration of six flavourings under heating conditions and their effects on the physical and chemical properties of aerosols[J]. Journal of Light Industry, 2021, 36(5): 67-75. doi: 10.12187/2021.05.009
    Citation:SI Xiaoxi, ZHANG Fengmei, ZHU Ruizhi, et al. Study on the release and migration of six flavourings under heating conditions and their effects on the physical and chemical properties of aerosols[J]. Journal of Light Industry, 2021, 36(5): 67-75.doi:10.12187/2021.05.009
    shu

    6种香料在加热条件下的释放迁移及对气溶胶理化特性的影响

      作者简介:司晓喜(1986-),男,云南省昆明市人,云南中烟工业有限责任公司高级工程师,主要研究方向为烟草和烟气化学.
    • 1. 云南中烟工业有限责任公司 技术中心/云南省烟草化学重点实验室, 云南 昆明 650031;
    • 2. 中国烟草总公司郑州烟草研究院, 河南 郑州 450001
    • 收稿日期: 2021-05-14
    基金项目:中国烟草总公司重大专项项目（110201901002（XX-02））；云南省科技厅科技项目（202001AU070005）；云南中烟工业有限责任公司科技项目（2020YL03）

    摘要:采用吸烟机抽吸，结合GC-MS/MS和快速粒径仪检测，研究了6种香料在加热条件下向烟气气溶胶的迁移及对气溶胶理化特性的影响.实验结果表明：1）6种香料在350℃加热条件下均以原型蒸发为主.2）6种香料在加热抽吸时的释放迁移呈现不同特征，其中异戊酸异戊酯和2，3，5-三甲基吡嗪分布于烟气气溶胶粒相物和气相物中，其他4种香料均只分布于粒相物中；香叶醇和2-乙酰基吡咯向烟气气溶胶迁移的总迁移率为2.8%~8.1%，其余4种香料为17.6%~54.4%.3）与空白对照样相比，添加5%的L-薄荷醇或1%、2%的WS-23后，使烟碱、丙二醇和丙三醇向烟气气溶胶中的释放量降低了20%以上，在滤嘴段的截留量降低了10%以上.4）当L-薄荷醇添加量达5%时，气溶胶粒数浓度降低了28%、粒数中值直径（CMD）增大了8%.

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